Molecular Understanding of Reactivity and Selectivity for Methanol Oxidation at the Au/TiO 2  Interface | Zendy

Farnesi Camellone Matteo | Zendy; Zhao Jianli | Zendy; Jin Lanying | Zendy; Wang Yuemin | Zendy; Muhler Martin | Zendy; Marx Dominik | Zendy

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Molecular Understanding of Reactivity and Selectivity for Methanol Oxidation at the Au/TiO 2 Interface

Author(s) -

Farnesi Camellone Matteo,

Zhao Jianli,

Jin Lanying,

Wang Yuemin,

Muhler Martin,

Marx Dominik

Publication year - 2013

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201301868

Subject(s) - reactivity (psychology) , catalysis , methanol , interface (matter) , formaldehyde , selectivity , service (business) , computer science , chemistry , nanotechnology , database , materials science , molecule , organic chemistry , business , medicine , gibbs isotherm , alternative medicine , pathology , marketing

Gold catalysis : Experimental and theoretical data demonstrated consistently that the interfacial sites on a Au/TiO 2 catalyst show both high reactivity and selectivity for low‐temperature methanol oxidation with O 2 to give formaldehyde. The microscopic mechanism of this complex reaction has been unraveled in full molecular detail (see picture, gold cluster on TiO 2 surface).

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