Pulling the Levers of Photophysics: How Structure Controls the Rate of Energy Dissipation | Zendy

Kuhlman Thomas S. | Zendy; Pittelkow Michael | Zendy; Sølling Theis I. | Zendy; Møller Klaus B. | Zendy

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Pulling the Levers of Photophysics: How Structure Controls the Rate of Energy Dissipation

Author(s) -

Kuhlman Thomas S.,

Pittelkow Michael,

Sølling Theis I.,

Møller Klaus B.

Publication year - 2013

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201208197

Subject(s) - dissipation , adiabatic process , energy (signal processing) , computer science , statistical physics , service (business) , physics , information retrieval , thermodynamics , quantum mechanics , business , marketing

Internal conversion : The energy difference between the Franck–Condon and equilibrium geometries and the vibrational frequency of one or a few modes determine the relative importance of adiabatic and nonadiabatic dynamics and thus the rate of electronic energy dissipation (see picture). In the cycloketones, variations in these quantities lead to a difference in the timescale for the S 2 →S 1 transition.

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