Production of  p ‐Xylene from Biomass by Catalytic Fast Pyrolysis Using ZSM‐5 Catalysts with Reduced Pore Openings | Zendy

Cheng YuTing | Zendy; Wang Zhuopeng | Zendy; Gilbert Christopher J. | Zendy; Fan Wei | Zendy; Huber George W. | Zendy

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Production of p ‐Xylene from Biomass by Catalytic Fast Pyrolysis Using ZSM‐5 Catalysts with Reduced Pore Openings

Author(s) -

Cheng YuTing,

Wang Zhuopeng,

Gilbert Christopher J.,

Fan Wei,

Huber George W.

Publication year - 2012

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201205230

Subject(s) - pyrolysis , catalysis , selectivity , zsm 5 , xylene , furan , biomass (ecology) , chemical engineering , chemistry , organic chemistry , zeolite , materials science , toluene , geology , engineering , oceanography

Pores for thought : Chemical liquid deposition of silica onto ZSM‐5 catalysts led to smaller pore openings that resulted in >90 % selectivity for p ‐xylene over the other xylenes in the catalytic fast pyrolysis of furan and 2‐methylfuran (see scheme). The p‐ xylene selectivity increased from 51 % with gallium spray‐dried ZSM‐5 to 72 % with a pore‐mouth‐modified catalyst in the pyrolysis of pine wood.

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