Hydrogenation of Carbon Dioxide to Methanol by Using a Homogeneous Ruthenium–Phosphine Catalyst | Zendy

Wesselbaum Sebastian | Zendy; vom Stein Thorsten | Zendy; Klankermayer Jürgen | Zendy; Leitner Walter | Zendy

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Hydrogenation of Carbon Dioxide to Methanol by Using a Homogeneous Ruthenium–Phosphine Catalyst

Author(s) -

Wesselbaum Sebastian,

vom Stein Thorsten,

Klankermayer Jürgen,

Leitner Walter

Publication year - 2012

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201202320

Subject(s) - phosphine , ruthenium , homogeneous , methanol , catalysis , carbon dioxide , chemistry , homogeneous catalysis , organic chemistry , chemical engineering , physics , engineering , thermodynamics

Simply efficient : The homogenously catalyzed hydrogenation of CO 2 to methanol is achieved by using a ruthenium phosphine complex under relatively mild conditions (see scheme; HNTf 2 =bis(trifluoromethane)sulfonimide). This is the first example of CO 2 hydrogenation to methanol by using a single molecularly defined catalyst.

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