Incarceration of (PdO)  n   and Pd  n   Clusters by Cage‐Templated Synthesis of Hollow Silica Nanoparticles | Zendy

Takao Kiyotaka | Zendy; Suzuki Kosuke | Zendy; Ichijo Tatsuya | Zendy; Sato Sota | Zendy; Asakura Hiroyuki | Zendy; Teramura Kentaro | Zendy; Kato Kazuo | Zendy; Ohba Tomonori | Zendy; Morita Takeshi | Zendy; Fujita Makoto | Zendy

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Incarceration of (PdO) n and Pd n Clusters by Cage‐Templated Synthesis of Hollow Silica Nanoparticles

Author(s) -

Takao Kiyotaka,

Suzuki Kosuke,

Ichijo Tatsuya,

Sato Sota,

Asakura Hiroyuki,

Teramura Kentaro,

Kato Kazuo,

Ohba Tomonori,

Morita Takeshi,

Fujita Makoto

Publication year - 2012

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201201288

Subject(s) - nanoparticle , palladium , metal , materials science , nanotechnology , cage , oxide , silicon dioxide , chemical engineering , chemistry , catalysis , crystallography , organic chemistry , metallurgy , mathematics , combinatorics , engineering

Imprisoned palladium : A unique approach is developed to incarcerate metal clusters with strictly controlled n values within hollow silica nanoparticles. A Pd 12 L 24 spherical complex is used as a template for the hollow silica synthesis. The incarcerated Pd 12 L 24 core is calcinated to give (PdO) n oxide clusters and subsequently reduced to Pd n metal clusters within the protective hollow silica.

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