Analysis of the Broadening of X‐ray Photoelectron Spectroscopy Peaks for Ionic Crystals | Zendy

Nelin Connie J. | Zendy; Bagus Paul S. | Zendy; Brown Matthew A. | Zendy; Sterrer Martin | Zendy; Freund HansJoachim | Zendy

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Analysis of the Broadening of X‐ray Photoelectron Spectroscopy Peaks for Ionic Crystals

Author(s) -

Nelin Connie J.,

Bagus Paul S.,

Brown Matthew A.,

Sterrer Martin,

Freund HansJoachim

Publication year - 2011

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.201100964

Subject(s) - x ray photoelectron spectroscopy , ionic bonding , monolayer , ionization , spectral line , oxide , x ray , chemistry , spectroscopy , bond length , crystallography , atomic physics , materials science , physics , nuclear magnetic resonance , nanotechnology , crystal structure , optics , ion , quantum mechanics , organic chemistry

Breathing : A simple and intuitive approach relates changes in bond lengths of core‐hole ionized states to the extent of vibrational fine structure, or Franck–Condon broadening (Δ E ), in X‐ray photoelectron spectra of ionic compounds. For the extreme case of a monolayer of MgO on Ag(100), the difference in Franck–Condon broadening compared to bulk MgO reflects the different binding situation in the supported oxide (see picture, r =MgO distance).

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