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Premium Peculiar Nonmonotonic Water Incorporation in Oxides Detected by Local In Situ Optical Absorption Spectroscopy
Author(s)
Yu Ji Haeng,
Lee JongSook,
Maier Joachim
Publication year2007
Publication title
angewandte chemie international edition
Resource typeJournals
PublisherWILEY‐VCH Verlag
Hydrogen first, oxygen next : The kinetics of water incorporation in situ has been followed by spatially resolved local optical absorption spectroscopy as well as by integral conductance by using SrTiO 3 as a model oxide proton conductor. The surprising nonmonotonic redox kinetics can be explained by a decoupling of the H 2 O diffusion into a fast diffusion of hydrogen and a more sluggish diffusion of oxygen (see picture).
Subject(s)absorption (acoustics) , absorption spectroscopy , analytical chemistry (journal) , chemical physics , chemistry , composite material , control engineering , decoupling (probability) , diffusion , engineering , hydrogen , in situ , kinetics , materials science , optics , organic chemistry , oxide , oxygen , photochemistry , physics , proton , quantum mechanics , spectroscopy , thermodynamics
Language(s)English
SCImago Journal Rank5.831
H-Index550
eISSN1521-3773
pISSN1433-7851
DOI10.1002/anie.200701765

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