Broadband Femtosecond Fluorescence Spectroscopy of [Ru(bpy) 3 ] 2+ | Zendy

Cannizzo Andrea | Zendy; van Mourik Frank | Zendy; Gawelda Wojciech | Zendy; Zgrablic Goran | Zendy; Bressler Christian | Zendy; Chergui Majed | Zendy

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Broadband Femtosecond Fluorescence Spectroscopy of [Ru(bpy) 3 ] 2+

Author(s) -

Cannizzo Andrea,

van Mourik Frank,

Gawelda Wojciech,

Zgrablic Goran,

Bressler Christian,

Chergui Majed

Publication year - 2006

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.200600125

Subject(s) - intersystem crossing , femtosecond , photon upconversion , spectroscopy , luminescence , singlet state , fluorescence , energy transfer , ultrashort pulse , chemistry , photochemistry , fluorescence spectroscopy , ultrafast laser spectroscopy , analytical chemistry (journal) , excited state , atomic physics , materials science , physics , optoelectronics , molecular physics , optics , laser , quantum mechanics , chromatography

It's sizzling! Femtosecond fluorescence‐upconversion studies of aqueous [Ru(bpy) 3 ] 2+ show a short‐lived vibrationally hot emission of the singlet metal‐to‐ligand charge‐transfer state, with an ultrafast intersystem crossing (≈10 fs) to the triplet state at constant energy (the colors indicate the luminescence intensity).

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