Dysprosium Triangles Showing Single‐Molecule Magnet Behavior of Thermally Excited Spin States | Zendy

Tang Jinkui | Zendy; Hewitt Ian | Zendy; Madhu N. T. | Zendy; Chastanet Guillaume | Zendy; Wernsdorfer Wolfgang | Zendy; Anson Christopher E. | Zendy; Benelli Cristiano | Zendy; Sessoli Roberta | Zendy; Powell Annie K. | Zendy

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Dysprosium Triangles Showing Single‐Molecule Magnet Behavior of Thermally Excited Spin States

Author(s) -

Tang Jinkui,

Hewitt Ian,

Madhu N. T.,

Chastanet Guillaume,

Wernsdorfer Wolfgang,

Anson Christopher E.,

Benelli Cristiano,

Sessoli Roberta,

Powell Annie K.

Publication year - 2006

Publication title -

angewandte chemie international edition

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 5.831

H-Index - 550

eISSN - 1521-3773

pISSN - 1433-7851

DOI - 10.1002/anie.200503564

Subject(s) - dysprosium , excited state , single molecule magnet , unpaired electron , magnet , ground state , spin (aerodynamics) , electron , condensed matter physics , molecule , atomic physics , materials science , physics , chemistry , magnetic field , magnetization , quantum mechanics , inorganic chemistry , thermodynamics

Roll the Dy's : Two aggregates made up of dysprosium triangles (one example is shown) display a vanishing susceptibility at low temperature, unprecedented in systems comprising an odd number of unpaired electrons. Despite having a near non‐magnetic ground state, behavior typical of a single‐molecule magnet is observed for the thermally populated excited state.

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