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Alkenylcarbene Ruthenium Arene Complexes as Initiators of Alkene Metathesis: An Enyne Creates a Catalyst that Promotes Its Selective Transformation
Author(s) -
Castarlenas Ricardo,
Eckert Matthieu,
Dixneuf Pierre H.
Publication year - 2005
Publication title -
angewandte chemie
Language(s) - German
Resource type - Journals
eISSN - 1521-3757
pISSN - 0044-8249
DOI - 10.1002/ange.200462865
Subject(s) - alkene , metathesis , ruthenium , chemistry , catalysis , enyne metathesis , enyne , stereochemistry , transformation (genetics) , combinatorial chemistry , organic chemistry , polymer , polymerization , biochemistry , gene
Ein Molekül erzeugt seinen Katalysator : [RuCl(aren)(PCy 3 )]OTf (z. B. 1 ) erzeugt mit Allyl‐ oder Propylpropargylethern in einer Metallo‐retro‐En‐Reaktion die Alkenylcarben‐Derivate 2 . Diese effizienten Ringschlussmetathese‐Katalysatoren wandeln Allylpropargylether in Alkenylcycloalkene und Diene in cyclische Alkene um (siehe Schema).

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