Stable Cycling of Lithium Metal Batteries Using High Transference Number Electrolytes | Zendy

Lu Yingying | Zendy; Tikekar Mukul | Zendy; Mohanty Ritesh | Zendy; Hendrickson Kenville | Zendy; Ma Lin | Zendy; Archer Lynden A. | Zendy

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Stable Cycling of Lithium Metal Batteries Using High Transference Number Electrolytes

Author(s) -

Lu Yingying,

Tikekar Mukul,

Mohanty Ritesh,

Hendrickson Kenville,

Ma Lin,

Archer Lynden A.

Publication year - 2015

Publication title -

advanced energy materials

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 10.08

H-Index - 220

eISSN - 1614-6840

pISSN - 1614-6832

DOI - 10.1002/aenm.201402073

Subject(s) - electrolyte , lithium (medication) , lithium metal , materials science , electrical conductor , membrane , metal , nanotechnology , chemical engineering , chemistry , electrode , composite material , metallurgy , engineering , medicine , endocrinology , biochemistry

An electrolyte with high lithium transference number ( t Li+ ) is predicted by theory to retard lithium dendrite formation and growth in rechargeable lithium metal batteries. Lithiated perfluorinated polymer electrolyte membranes (Li‐PEM) are synthesized to study the effects of t Li+ on Li dendrite growth in an ideally single‐ion conductive electrolyte system. Consistent with theory, a more than 40‐fold improvement in cell lifetime is found.

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