Open AccessIntrinsically Stretchable Organic Electrochemical Transistors with Rigid‐Device‐Benchmarkable Performance
Author(s) -
Liu Dingyao,
Tian Xinyu,
Bai Jing,
Wang Yan,
Cheng Yixun,
Ning Weijie,
Chan Paddy K. L.,
Wu Kai,
Sun Junqi,
Zhang Shiming
Publication year - 2022
Publication title -
advanced science
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 5.388
H-Index - 100
ISSN - 2198-3844
DOI - 10.1002/advs.202203418
Subject(s) - interfacing , stretchable electronics , nanotechnology , materials science , transistor , neuromorphic engineering , substrate (aquarium) , soft materials , electronics , optoelectronics , computer science , electrical engineering , computer hardware , engineering , oceanography , voltage , machine learning , geology , artificial neural network
Intrinsically stretchable organic electrochemical transistors (OECTs) are being pursued as the next‐generation tissue‐like bioelectronic technologies to improve the interfacing with the soft human body. However, the performance of current intrinsically stretchable OECTs is far inferior to their rigid counterparts. In this work, for the first time, the authors report intrinsically stretchable OECTs with overall performance benchmarkable to conventional rigid devices. In particular, oxygen level in the stretchable substrate is revealed to have a significant impact on the on/off ratio. By employing stretchable substrates with low oxygen permeabilities, the on/off ratio is elevated from ≈10 to a record‐high value of ≈10 4 , which is on par with a rigid OECT. The device remained functional after cyclic stretching tests. This work demonstrates that intrinsically stretchable OECTs have the potential to serve as a new building block for emerging soft bioelectronic applications such as electronic skin, soft implantables, and soft neuromorphic computing.