Oxidative Coupling between Methylarenes and Ammonia: A Direct Approach to Aromatic Primary Amides | Zendy

Zhao Zhenguang | Zendy; Wang Tao | Zendy; Yuan Lin | Zendy; Hu Xu | Zendy; Xiong Fei | Zendy; Zhao Junfeng | Zendy

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Oxidative Coupling between Methylarenes and Ammonia: A Direct Approach to Aromatic Primary Amides

Author(s) -

Zhao Zhenguang,

Wang Tao,

Yuan Lin,

Hu Xu,

Xiong Fei,

Zhao Junfeng

Publication year - 2015

Publication title -

advanced synthesis and catalysis

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.541

H-Index - 155

eISSN - 1615-4169

pISSN - 1615-4150

DOI - 10.1002/adsc.201500310

Subject(s) - chemistry , primary (astronomy) , ammonia , oxidative coupling of methane , catalysis , aqueous solution , oxidative phosphorylation , chloride , iodide , organic chemistry , surface modification , coupling (piping) , combinatorial chemistry , mechanical engineering , biochemistry , physics , astronomy , engineering

A direct oxidative amidation between methylarenes and aqueous ammonia using a tert ‐butyl hydroperoxide and tetrabutylammonium iodide (TBHP/TBAI) oxidation system with co‐catalysis of iron(III) chloride has been developed. Both coupling partners were used in their native form to render prior functionalization unnecessary and afford a facile approach to aromatic primary amides.

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