Heterogeneous or Homogeneous? A Case Study Involving Palladium‐Containing Perovskites in the Suzuki Reaction | Zendy

Andrews Stephen P. | Zendy; Stepan Antonia F. | Zendy; Tanaka Hirohisa | Zendy; Ley Steven V. | Zendy; Smith Martin D. | Zendy

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Heterogeneous or Homogeneous? A Case Study Involving Palladium‐Containing Perovskites in the Suzuki Reaction

Author(s) -

Andrews Stephen P.,

Stepan Antonia F.,

Tanaka Hirohisa,

Ley Steven V.,

Smith Martin D.

Publication year - 2005

Publication title -

advanced synthesis and catalysis

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.541

H-Index - 155

eISSN - 1615-4169

pISSN - 1615-4150

DOI - 10.1002/adsc.200404331

Subject(s) - chemistry , palladium , catalysis , homogeneous , perovskite (structure) , phase (matter) , heterogeneous catalysis , kinetic energy , homogeneous catalysis , suzuki reaction , chemical engineering , organic chemistry , thermodynamics , physics , quantum mechanics , engineering

The utility of a series of palladium‐containing perovskite catalysts in the Suzuki reaction is described; turnover numbers of up to 400,000 are reported. A detailed investigation into the mode of action of these catalysts encompassing kinetic studies, catalyst poisoning, microscopy and three‐phase tests demonstrate that these heterogeneous materials are pre‐catalysts that operate by a solution‐phase mechanism

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