Ultra‐thin Solid‐State Li‐Ion Electrolyte Membrane Facilitated by a Self‐Healing Polymer Matrix | Zendy

Whiteley Justin M. | Zendy; Taynton Philip | Zendy; Zhang Wei | Zendy; Lee SeHee | Zendy

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Ultra‐thin Solid‐State Li‐Ion Electrolyte Membrane Facilitated by a Self‐Healing Polymer Matrix

Author(s) -

Whiteley Justin M.,

Taynton Philip,

Zhang Wei,

Lee SeHee

Publication year - 2015

Publication title -

advanced materials

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 10.707

H-Index - 527

eISSN - 1521-4095

pISSN - 0935-9648

DOI - 10.1002/adma.201502636

Subject(s) - materials science , membrane , polymer , separator (oil production) , electrolyte , solid state , nanotechnology , computer science , composite material , engineering physics , engineering , physics , electrode , thermodynamics , genetics , biology , quantum mechanics

Thin solid membranes are formed by a new strategy, whereby an in situ derived self‐healing polymer matrix that penetrates the void space of an inorganic solid is created. The concept is applied as a separator in an all‐solid‐state battery with an FeS 2 ‐based cathode and achieves tremendous performance for over 200 cycles. Processing in dry conditions represents a paradigm shift for incorporating high active‐material mass loadings into mixed‐matrix membranes.

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