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Structure Inversion Asymmetry and Rashba Effect in Quantum Confined Topological Crystalline Insulator Heterostructures
Author(s) -
Rechciński Rafał,
Galicka Marta,
Simma Mathias,
Volobuev Valentine V.,
Caha Ondřej,
SánchezBarriga Jaime,
Mandal Partha S.,
Golias Evangelos,
Varykhalov Andrei,
Rader Oliver,
Bauer Günther,
Kacman Perła,
Buczko Ryszard,
Springholz Gunther
Publication year - 2021
Publication title -
advanced functional materials
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 6.069
H-Index - 322
eISSN - 1616-3028
pISSN - 1616-301X
DOI - 10.1002/adfm.202008885
Subject(s) - topological insulator , asymmetry , heterojunction , condensed matter physics , surface states , point reflection , electronic structure , rashba effect , electronic band structure , quantum well , materials science , physics , position and momentum space , topology (electrical circuits) , surface (topology) , quantum mechanics , spintronics , geometry , laser , mathematics , ferromagnetism , combinatorics
Structure inversion asymmetry is an inherent feature of quantum confined heterostructures with non‐equivalent interfaces. It leads to a spin splitting of the electron states and strongly affects the electronic band structure. The effect is particularly large in topological insulators because the topological surface states are extremely sensitive to the interfaces. Here, the first experimental observation and theoretical explication of this effect are reported for topological crystalline insulator quantum wells made of Pb 1− x Sn x Se confined by Pb 1− y Eu y Se barriers on one side and by vacuum on the other. This provides a well defined structure asymmetry controlled by the surface condition. The electronic structure is mapped out by angle‐resolved photoemission spectroscopy and tight binding calculations, evidencing that the spin splitting decisively depends on hybridization and, thus, quantum well width. Most importantly, the topological boundary states are not only split in energy but also separated in space—unlike conventional Rashba bands that are splitted only in momentum. The splitting can be strongly enhanced to very large values by control of the surface termination due to the charge imbalance at the polar quantum well surface. The findings thus, open up a wide parameter space for tuning of such systems for device applications.