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Ultrahigh Speed and Broadband Few‐Layer MoTe 2 /Si 2D–3D Heterojunction‐Based Photodiodes Fabricated by Pulsed Laser Deposition
Author(s) -
Lu Zhijian,
Xu Yan,
Yu Yongqiang,
Xu Kewei,
Mao Jie,
Xu Gaobin,
Ma Yuanming,
Wu Di,
Jie Jiansheng
Publication year - 2020
Publication title -
advanced functional materials
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 6.069
H-Index - 322
eISSN - 1616-3028
pISSN - 1616-301X
DOI - 10.1002/adfm.201907951
Subject(s) - materials science , photodiode , heterojunction , optoelectronics , responsivity , photodetector , fabrication , specific detectivity , laser , broadband , ultrashort pulse , pulsed laser deposition , thin film , optics , nanotechnology , physics , medicine , alternative medicine , pathology
2D transition metal dichalcogenides are promising candidates for high‐performance photodetectors. However, the relatively low response speed as well as the complex transfer process hinders their wide applications. Herein, for the first time, the fabrication of a few‐layer MoTe 2 /Si 2D–3D vertical heterojunction for high‐speed and broadband photodiodes by a pulsed laser deposition technique is reported. Owing to the high junction quality, ultrathin MoTe 2 film thickness, and unique vertical n–n heterojunction structure, the photodiode exhibits excellent device performance in terms of a high responsivity of 0.19 A W −1 and a large detectivity of 6.8 × 10 13 Jones. The device is also capable of detecting a broadband light with wavelength spanning from 300 to 1800 nm. More importantly, the device possesses an ultrahigh response speed up to 150 ns with a 3‐dB electrical bandwidth approaching 0.12 GHz. This work paves the way toward the fabrication of novel 2D–3D heterojunctions for high‐performance, ultrafast photodetectors.