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3D‐Printed All‐Fiber Li‐Ion Battery toward Wearable Energy Storage
Author(s) -
Wang Yibo,
Chen Chaoji,
Xie Hua,
Gao Tingting,
Yao Yonggang,
Pastel Glenn,
Han Xiaogang,
Li Yiju,
Zhao Jiupeng,
Fu Kun Kelvin,
Hu Liangbing
Publication year - 2017
Publication title -
advanced functional materials
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 6.069
H-Index - 322
eISSN - 1616-3028
pISSN - 1616-301X
DOI - 10.1002/adfm.201703140
Subject(s) - materials science , battery (electricity) , fiber , anode , flexibility (engineering) , nanotechnology , energy storage , cathode , electrolyte , wearable computer , lithium (medication) , lithium iron phosphate , electrode , wearable technology , fabrication , electrospinning , electrochemistry , polymer , computer science , composite material , electrical engineering , power (physics) , embedded system , physics , engineering , quantum mechanics , alternative medicine , mathematics , chemistry , endocrinology , pathology , medicine , statistics
Conventional bulky and rigid power systems are incapable of meeting flexibility and breathability requirements for wearable applications. Despite the tremendous efforts dedicated to developing various 1D energy storage devices with sufficient flexibility, challenges remain pertaining to fabrication scalability, cost, and efficiency. Here, a scalable, low‐cost, and high‐efficiency 3D printing technology is applied to fabricate a flexible all‐fiber lithium‐ion battery (LIB). Highly viscous polymer inks containing carbon nanotubes and either lithium iron phosphate (LFP) or lithium titanium oxide (LTO) are used to print LFP fiber cathodes and LTO fiber anodes, respectively. Both fiber electrodes demonstrate good flexibility and high electrochemical performance in half‐cell configurations. All‐fiber LIB can be successfully assembled by twisting the as‐printed LFP and LTO fibers together with gel polymer as the quasi‐solid electrolyte. The all‐fiber device exhibits a high specific capacity of ≈110 mAh g −1 at a current density of 50 mA g −1 and maintains a good flexibility of the fiber electrodes, which can be potentially integrated into textile fabrics for future wearable electronic applications.