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DMS role in ENSO cycle in the tropics
Author(s) -
Xu Li,
CameronSmith Philip,
Russell Lynn M.,
Ghan Steven J.,
Liu Ying,
Elliott Scott,
Yang Yang,
Lou Sijia,
Lamjiri Maryam A.,
Manizza Manfredi
Publication year - 2016
Publication title -
journal of geophysical research: atmospheres
Language(s) - English
Resource type - Journals
eISSN - 2169-8996
pISSN - 2169-897X
DOI - 10.1002/2016jd025333
Subject(s) - dimethyl sulfide , environmental science , climatology , atmospheric sciences , sulfate , sea surface temperature , el niño southern oscillation , aerosol , carbonyl sulfide , sulfur , meteorology , geology , chemistry , geography , organic chemistry
We examined the multiyear mean and variability of dimethyl sulfide (DMS) and its relationship to sulfate aerosols, as well as cloud microphysical and radiative properties. We conducted a 150 year simulation using preindustrial conditions produced by the Community Earth System Model embedded with a dynamic DMS module. The model simulated the mean spatial distribution of DMS emissions and burden, as well as sulfur budgets associated with DMS, SO 2 , H 2 SO 4 , and sulfate that were generally similar to available observations and inventories for a variety of regions. Changes in simulated sea‐to‐air DMS emissions and associated atmospheric abundance, along with associated aerosols and cloud and radiative properties, were consistently dominated by El Niño–Southern Oscillation (ENSO) cycle in the tropical Pacific region. Simulated DMS, aerosols, and clouds showed a weak positive feedback on sea surface temperature. This feedback suggests a link among DMS, aerosols, clouds, and climate on interannual timescales. The variability of DMS emissions associated with ENSO was primarily caused by a higher variation in wind speed during La Niña events. The simulation results also suggest that variations in DMS emissions increase the frequency of La Niña events but do not alter ENSO variability in terms of the standard deviation of the Niño 3 sea surface temperature anomalies.