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Nitrile imines generated by the oxidative dehydrogenation of aromatic aldehyde phenylhydrazones with chloramine-T as a catalytic dehydrogenating agent were trapped in situ by 4-methoxy cinnamonitrile to aord 3,4- diaryl-1-phenyl-4,5-dihydro- 1H -pyrazole-5-carbonitrile in moderate to good yields. The structures of the cycloadducts were conrmed by spectral studies and elemental analysis.

Synthesis of 3,4-diaryl-1-phenyl-4,5-dihydro-1$H$-pyrazole-5-carbonitriles via 1,3-dipolar cycloaddition reactions