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A Schiff base ligand derived from 4-(benzeneazo) salicylaldehyde and   (±)trans-1,2-cyclohexanediamine (H2L) and its corresponding Cu(II) complex   (CuL) has been synthesized and characterized by FT-IR, UV-VIS and 1H NMR. The   copper Schiff base complex encapsulated in the nanopores of zeolite-Y (CuL-Y)   by flexible ligand method and its encapsulation have been ensured by   different studies. The homogeneous and its corresponding heterogeneous   catalysts have been used for oxidation of different alkenes with tert-butyl   hydroperoxide. Under the optimized reaction conditions, the oxidation of   cyclooctene, cyclohexene, styrene and norbornene catalyzed by CuL gave 89,   63, 46 and 13% conversion, respectively. These olefins were oxidized   efficiently with 50, 96, 96 and 92% conversion in the presence of CuL-Y,   respectively. Comparison of the catalytic behavior of CuL and CuL-Y showed   the higher catalytic activity and selectivity of the heterogeneous catalyst   with respect to the homogenous one

journal of the serbian chemical society

Copper(II) complex of (±)trans-1,2-cyclohexanediamine azo-linked Schiff base ligand encapsulated in nanocavity of zeolite-Y for the catalytic oxidation of olefins