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In order to explore new more powerful ultrashort pulse laser and tunable laser for diode-pumping, this paper reports the growth and spectral assessment of Yb 3+ -doped KBaGd(MoO 4 ) 3  crystal. An Yb 3+ :KBaGd(MoO 4 ) 3  crystal with dimensions of 50×40×9 mm 3  was grown by the TSSG method from the K 2 Mo 2 O 7  flux. The investigated spectral properties indicated that Yb 3+ :KBaGd(MoO 4 ) 3  crystal exhibits broad absorption and emission bands, except the large emission and gain cross-sections. This feature of the broad absorption and emission bands is not only suitable for the diode pumping, but also for the production of ultrashort pulses and tunability. Therefore, Yb 3+ :KBaGd(MoO 4 ) 3  crystal can be regarded as a candidate for the ultrashort pulse and tunable lasers.

Growth and Spectral Assessment of Yb3+-Doped KBaGd(MoO4)3 Crystal: A Candidate for Ultrashort Pulse and Tunable Lasers