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Two-beam coupling by nitrogen-vacancy centers in diamond
Author(s) -
D. A. Redman,
Q. Z. Shu,
Alan Lenef,
S. C. Rand
Publication year - 1992
Publication title -
optics letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.524
H-Index - 272
eISSN - 1071-2763
pISSN - 0146-9592
DOI - 10.1364/ol.17.000175
Subject(s) - diamond , excited state , materials science , optics , grating , refractive index , vacancy defect , intersystem crossing , beam (structure) , coupling (piping) , atomic physics , molecular physics , condensed matter physics , optoelectronics , physics , singlet state , metallurgy , composite material
A new method for two-beam coupling measurements based on acousto-optic modulation with subhertz tuning capability is applied to study excited-state dynamics of the nitrogen-vacancy center in diamond. Results yield fundamental decay constants and the nonlinear refractive index and are in good agreement with the calculated dual grating response to resonances in the microscopic susceptibility due to intersystem crossing and spin-lattice relaxation.

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