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Picosecond time-resolved four-wave mixing experiments in sodium-seeded flames
Author(s) -
John T. Fourkas,
Timothy R. Brewer,
Hackjin Kim,
M. D. Fayer
Publication year - 1991
Publication title -
optics letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.524
H-Index - 272
eISSN - 1071-2763
pISSN - 0146-9592
DOI - 10.1364/ol.16.000177
Subject(s) - picosecond , materials science , excited state , atomic physics , optics , four wave mixing , population , polarization (electrochemistry) , mixing (physics) , coherence (philosophical gambling strategy) , physics , nonlinear optics , chemistry , laser , demography , quantum mechanics , sociology
Picosecond four-wave mixing experiments have been used to study collisions in a Na-seeded, premixed, methane-air flame. Population gratings are used to measure Na excited-state quenching collision rates, while polarization gratings are used to measure Na ground-state hyperfine coherence randomizing collision rates and overall Na diffusion rates, even though these processes are slower than the excited-state quenching rate.

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