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Self-consistent dielectric constant determination for monolayer WSe2
Author(s) -
SeongYeon Lee,
TaeYoung Jeong,
JiHee Kim,
Seokjoon Yun,
KiJu Yee
Publication year - 2018
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.26.023061
Subject(s) - exciton , monolayer , dielectric , trion , materials science , spectral line , dispersion (optics) , condensed matter physics , transmittance , coupling constant , optics , dispersion relation , kramers–kronig relations , molecular physics , atomic physics , refractive index , physics , optoelectronics , nanotechnology , astronomy , particle physics
Frequency-dependent dielectric constant dispersion of monolayer WSe 2 , ε(ω)=ε 1 (ω)+i ε 2 (ω), was obtained from simultaneously measured transmittance and reflectance spectra. Optical transitions of the trion as well as A-, B-, and C-excitons are clearly resolved in the  ε 2 spectrum. A consistent Kramers-Kronig transformation between the ε 1 and  ε 2 spectra support the validity of the applied analysis. It is found that the A- and B-exciton splitting in the case of the double-layer WSe 2 can be attributed to the spin-orbit coupling, which is larger than that in the monolayer WSe 2 . In addition, the temperature-induced evolution of the A-exciton energy and its width are explained by model equations with electron-phonon interactions.

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