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Doppler-free spectroscopy with a terahertz quantum-cascade laser
Author(s) -
M. Wienold,
Tasmim Alam,
L. Schrottke,
H. T. Grahn,
H.-W. Hübers
Publication year - 2018
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.26.006692
Subject(s) - laser linewidth , quantum cascade laser , optics , spectroscopy , cascade , doppler effect , terahertz radiation , laser , absorption spectroscopy , materials science , free spectral range , physics , chemistry , chromatography , quantum mechanics , astronomy
We report on the Doppler-free saturation spectroscopy of a molecular transition at 3.3 THz based on a quantum-cascade laser and an absorption cell in a collinear pump-probe configuration. A Lamb dip with a sub-Doppler linewidth of 170 kHz is observed for a rotational transition of HDO. We found that a certain level of external optical feedback is tolerable as long as the free spectral range of the external cavity is large compared to the width of the absorption line.

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