Frequency modulation spectroscopy with a THz quantum-cascade laser
Author(s) -
R. Eichholz,
Heiko Richter,
M. Wienold,
L. Schrottke,
R. Hey,
H. T. Grahn,
H.-W. Hübers
Publication year - 2013
Publication title -
optics express
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.394
H-Index - 271
ISSN - 1094-4087
DOI - 10.1364/oe.21.032199
Subject(s) - laser , quantum cascade laser , optics , frequency modulation , amplitude modulation , modulation (music) , materials science , terahertz radiation , spectroscopy , terahertz spectroscopy and technology , cascade , amplitude , pulse frequency modulation , dispersion (optics) , physics , pulse amplitude modulation , radio frequency , chemistry , pulse (music) , telecommunications , detector , chromatography , quantum mechanics , computer science , acoustics
We report on a terahertz spectrometer for high-resolution molecular spectroscopy based on a quantum-cascade laser. High-frequency modulation (up to 50 MHz) of the laser driving current produces a simultaneous modulation of the frequency and amplitude of the laser output. The modulation generates sidebands, which are symmetrically positioned with respect to the laser carrier frequency. The molecular transition is probed by scanning the sidebands across it. In this way, the absorption and the dispersion caused by the molecular transition are measured. The signals are modeled by taking into account the simultaneous modulation of the frequency and amplitude of the laser emission. This allows for the determination of the strength of the frequency as well as amplitude modulation of the laser and of molecular parameters such as pressure broadening.
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