The Spectrum of the Molecular Eigenstates of Pyrazine and the Reconstruction of Decays of Rotational States of the 1B3u (0–0) Transition of Pyrazine | Zendy

B.J. van der Meer | Zendy; Harry T. Jonkman | Zendy; Jan Kommandeur | Zendy

Open Access

The Spectrum of the Molecular Eigenstates of Pyrazine and the Reconstruction of Decays of Rotational States of the ¹B_3u (0–0) Transition of Pyrazine

Author(s) -

B.J. van der Meer,

Harry T. Jonkman,

Jan Kommandeur

Publication year - 1983

Publication title -

laser chemistry

Language(s) - English

Resource type - Journals

eISSN - 1026-8014

pISSN - 0278-6273

DOI - 10.1155/lc.2.77

Subject(s) - pyrazine , spectrum (functional analysis) , eigenvalues and eigenvectors , physics , chemistry , quantum mechanics , stereochemistry

The spectrum of the molecular eigenstates (ME) belonging to the various rotational members of the 1B3u (0-0) transition of pyrazine was measured with a very narrow band laser in a molecular beam with a Doppler width of 30 MHz. It is shown that, when the ME’s belonging to a single rotational state are Fourier-transformed, the beating decays of these states are obtained. A problem is constituted by the lack of a fast component in these reconstructions, while it is observed in experiments on higher J-states

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