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The spectrum of the molecular eigenstates (ME) belonging to the various rotational members of the 1B3u (0-0) transition of pyrazine was measured with a very narrow band laser in a molecular beam with a Doppler width of 30 MHz. It is shown that, when the ME’s belonging to a single rotational state are Fourier-transformed, the beating decays of these states are obtained. A problem is constituted by the lack of a fast component in these reconstructions, while it is observed in experiments on higher J-states

laser chemistry

The Spectrum of the Molecular Eigenstates of Pyrazine and the Reconstruction of Decays of Rotational States of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msup><mml:mi /><mml:mn>1</mml:mn></mml:msup><mml:msub><mml:mi>B</mml:mi><mml:mrow><mml:mn>3</mml:mn><mml:mi>u</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math> (0–0) Transition of Pyrazine

The Spectrum of the Molecular Eigenstates of Pyrazine and the Reconstruction of Decays of Rotational States of the 1B3u (0–0) Transition of Pyrazine