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CO in a supersonic pulsed beam is excited to the d3Δi state by VUV photons generated in a nonlinear four-wave mixing scheme. An excitation spectrum of the CO d3Δi (ν′ = 20, J′ = 1–3) is obtained at a resolution of 0.8 cm−1 for the first time. The radiative lifetimes of the rotational states are measured as 1.70 ± 0.08 μs, which are similar to but shorter than the lifetimes associated with lower vibrational levels.

laser chemistry

Laser Excitation Spectra and Lifetime Measurements of the CO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>d</mml:mi></mml:math>(<sup>3</sup>Δ<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mn /><mml:mi>i</mml:mi></mml:msub></mml:math>) State

Laser Excitation Spectra and Lifetime Measurements of the CO d(3Δi) State

Laser Excitation Spectra and Lifetime Measurements of the CO d(³Δi) State