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In this work photodissociation studies of glyoxal-H 2  (D 2 ) molecules have been conducted in order to analyze the effect of the mass in the vibrational predissociation of van der Waalscomplexes. The glyoxal-H 2  (D 2 ) molecules have been formed in a supersonic expansion andphotodissociated by means of a tunable dye laser. The final state of the glyoxal fragmentshas been determined by the analysis of the fluorescence spectrum. A significant isotope effecton the branching ratios for predissociation has been found. An interpretation in terms of adistorted wave diabatic treatment is presented.

Isotope Effect in the Vibrational Predissociation of van der Waals Molecules: Complexes of Glyoxal With H2 and D2