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Fine structures of 8-G-1-( p -YC 6 H 4 C ≡ CSe)C 10 H 6  [ 1  (G = H) and  2  (G = Cl): Y = H ( a ), OMe ( b ), Me ( c ), F ( d ), Cl ( e ), CN ( f ), and NO 2  ( g )] are determined by the X-ray analysis. Structures of  1 ,  2 , and  3  (G = Br) are called  A  if each Se–C sp  bond is perpendicular to the naphthyl plane, whereas they are  B  when the bond is placed on the plane. Structures are observed as  A  for  1a – c  bearing Y of nonacceptors, whereas they are  B  for  1e – g  with Y of strong acceptors. The change in the structures of  1e – g  versus those of  1a – c  is called Y-dependence in  1 . The Y-dependence is very specific in  1  relative to 1-( p -YC 6 H 4 Se)C 10 H 7  ( 4 ) due to the ethynyl group: the Y-dependence in  1  is almost inverse to the case of  4  due to the ethynyl group. We call the specific effect “ Ethynyl Influence. ” Structures of  2  are observed as  B : the  A -type structure of  1b  changes dramatically to  B  of  2b  by G = Cl at the 8-position, which is called G-dependence. The structures of  2  and  3  are examined in solutions based on the NMR parameters.

bioinorganic chemistry and applications/bioinorganic chemistry and applications

Fine Structures of 8-G-1-(<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>p</mml:mi></mml:math>-YC6H4C ≡ CSe)C10H6(G = H, Cl, and Br) in Crystals and Solutions: Ethynyl Influence and Y- and G-Dependences

Fine Structures of 8-G-1-(p-YC6H4C ≡ CSe)C10H6(G = H, Cl, and Br) in Crystals and Solutions: Ethynyl Influence and Y- and G-Dependences

Fine Structures of 8-G-1-(p-YC₆H₄C ≡ CSe)C₁₀H₆(G = H, Cl, and Br) in Crystals and Solutions: Ethynyl Influence and Y- and G-Dependences