Vibrational Dynamics in Molecular Condensed Phases With The Clio Free Electron Laser | Zendy

Claudine Crépin | Zendy; Michel Broquier | Zendy; H. Dubost | Zendy; D. L′hermite | Zendy; A. Tramer | Zendy; J. P. Galaup | Zendy; J.M. Berset | Zendy; J.M. Ortéga | Zendy

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Vibrational Dynamics in Molecular Condensed Phases With The Clio Free Electron Laser

Author(s) -

Claudine Crépin,

Michel Broquier,

H. Dubost,

D. L′hermite,

A. Tramer,

J. P. Galaup,

J.M. Berset,

J.M. Ortéga

Publication year - 1999

Publication title -

laser chemistry

Language(s) - English

Resource type - Journals

eISSN - 1026-8014

pISSN - 0278-6273

DOI - 10.1155/1999/95804

Subject(s) - chemistry , argon , absorption (acoustics) , echo (communications protocol) , electron , free electron model , laser , dynamics (music) , atomic physics , infrared , photon , analytical chemistry (journal) , molecular physics , optics , physics , computer network , organic chemistry , chromatography , computer science , acoustics , quantum mechanics

Single color pump-probe and photon-echo experiments have been performed on the COstretching mode of W(CO) 6 at about 1983 cm -1 in various liquids and solidenvironments. Combined with absorption data, the measured T 1 and T 2 times suggestthe following conclusions: in all liquids studied, the IR absorption band ishomogeneously broadened, whereas, inhomogeneous broadening is observed in solidmatrices and in a xerogel. At low temperature, the echo decay is much faster in methanethan in argon host.

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