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Single color pump-probe and photon-echo experiments have been performed on the COstretching mode of W(CO) 6   at about 1983 cm -1   in various liquids and solidenvironments. Combined with absorption data, the measured T 1   and T 2  times suggestthe following conclusions: in all liquids studied, the IR absorption band ishomogeneously broadened, whereas, inhomogeneous broadening is observed in solidmatrices and in a xerogel. At low temperature, the echo decay is much faster in methanethan in argon host.

Vibrational Dynamics in Molecular Condensed Phases With The Clio Free Electron Laser