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Intensity changes in Stokes resonance Raman spectra of photoexcited quaterphenyl arefound to result from 17 ps timescale changes in resonance frequency and width and alsoin Franck-Condon displacements. The 766 cm -1  anti-Stokes band shows a significanthot population which decays on a similar timescale. The results show that populationrelaxation, vibronic coupling and solvent reorganisation are all significant on thistimescale.

Picosecond Raman Excitation Profile and Transient Absorption Spectrum of S1 Quaterphenyl in Solution

Picosecond Raman Excitation Profile and Transient Absorption Spectrum of S₁ Quaterphenyl in Solution