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The carbonate radical (Co   3    −  ·) is of biological significance acting as an intermediate infree radical-mediated damage and is capable of oxidising amino acids and proteins. Inorder to distinguish between the four possible structures ofCo   3    −  ·, nanosecond timeresolvedresonance Raman (TR 3 ) experiments were undertaken. Photolysis ofpersulphate at 250 nm generated theSo   4    −  ·radical which then oxidised sodium carbonate.Resonance Raman spectra of the resultingCo   3    −  ·radical were obtained using a probewavelength of 620 nm. Point group theory calculations and interpretation of the TR 3 spectra suggest that the radical hasC   2  v molecular symmetry.

laser chemistry

The Carbonate, <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" id="E1"><mml:mrow><mml:msubsup><mml:mrow><mml:mtext>Co</mml:mtext></mml:mrow><mml:mtext>3</mml:mtext><mml:mrow><mml:msup><mml:mo>−</mml:mo><mml:mo>·</mml:mo></mml:msup></mml:mrow></mml:msubsup></mml:mrow></mml:math>, in Solution Studied by Resonance Raman Spectroscopy

The Carbonate, Co3−·, in Solution Studied by Resonance Raman Spectroscopy