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The reactions of Zn(4 1 P 1 ) with H 2  and D 2  were studied by employing a laser pump-and-probe technique. The nascent vibrational state distributions of ZnH(X  2∑  +    ) and ZnD(X  2∑  +    ) were determined. The distributions were much cooler than the statistically expected ones. These results are consistent with the insertive attack model proposed for other excited metal-H 2  systems. The quantum yield for the production of ZnH(X  2∑  +    ) was measured to be low; around 0.5 of that for cn4. Three-body dissociation processes to produce Zn(4 1 S 0 ) + H + H must be more dominant than the production of ZnH.

laser chemistry

Nascent Vibrational State Distributions of ZnH(X 2<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msup><mml:mo>∑</mml:mo><mml:mo>+</mml:mo></mml:msup></mml:mrow></mml:math> ) and ZnD(X 2<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msup><mml:mo>∑</mml:mo><mml:mo>+</mml:mo></mml:msup></mml:mrow></mml:math>) Produced in the Reactions of Zn(41P1) With H2 and D2

Nascent Vibrational State Distributions of ZnH(X 2∑+ ) and ZnD(X 2∑+) Produced in the Reactions of Zn(41P1) With H2 and D2

Nascent Vibrational State Distributions of ZnH(X ²∑+ ) and ZnD(X ²∑+) Produced in the Reactions of Zn(4¹P₁) With H₂ and D₂