Interfaces between Charged Surfaces and Ionic Liquids: Insights from Molecular Simulations | Zendy

Vladislav Ivaništšev | Zendy; Maxim V. Fedorov | Zendy

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Interfaces between Charged Surfaces and Ionic Liquids: Insights from Molecular Simulations

Author(s) -

Vladislav Ivaništšev,

Maxim V. Fedorov

Publication year - 2014

Publication title -

the electrochemical society interface

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 0.568

H-Index - 46

eISSN - 1944-8783

pISSN - 1064-8208

DOI - 10.1149/2.f08141if

Subject(s) - ion , chemical physics , monolayer , charge density , ionic liquid , ionic bonding , ionic potential , electrode , surface charge , layering , materials science , charge (physics) , chemistry , nanotechnology , physics , organic chemistry , botany , quantum mechanics , biology , catalysis

). However despite the many articles published on this subject (several hundred papers just in 2013) there is still no general agreement in the literature about the main factors that govern the structure and properties of ionic liquids at charged interfaces. This is mainly due to a large number of available combinations of ionic liquids (and their mixtures) and different surfaces. In this article, we make an attempt to rationalize recent experimental and computational findings on structural transitions in ionic liquids at charged interfaces. Herein, we present a critical (qualitative) analysis of available molecular modeling and experimental data using a recently developed concept of surface charge compensation that allows one to compare results for different ionic liquids on the same methodological footing. 6

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