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Core-level binding energies of all atoms are reported for the methyl substituted disilyl and digermyl chalcogenides, (Me n MH 3−n ) 2 E; where M = Si, Ge; E = O, S, Se, Te; n = 0, 1, 2, 3. Binding energies are also reported for the dimethyl series Me 2 E; where E = O, S, Se, Te; for the hydrides H 2 E; where E = O, S, Se; and for the methylhydrides MeEH; where E = O, S. Binding energy trends throughout these closely related series of compounds are discussed. The similarity of atomic charge patterns, deduced from the binding energies, for all molecules of a given silicon or germanium series are consistent with their ability to redistribute charge. The bonding mechanisms that make this possible are assessed.

ESCA investigations of Group IV derivatives. Part III. Binding energies for methyl substituted disilyl and digermyl chalcogenide series