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Emergent properties in transition metal oxide superlattices are traditionally tuned as functions of stoichiometry, reduced dimensionality, and epitaxial strain. Here the authors introduce a new tuning parameter, the connectivity of the $M$O${}_{6}$ octahedra ($M=$ transition metal), as a means to manipulate the electronic structure, symmetry, and competing ground states of oxide superlattices. They demonstrate this by the epitaxial growth of alternating layers of the high spin-orbit metal IrO${}_{2}$ and the band insulator TiO${}_{2}$, both of which have the rutile structure.

physical review materials

Rutile <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>IrO</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>TiO</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math> superlattices: A hyperconnected analog to the Ruddelsden-Popper structure

Rutile IrO2/TiO2 superlattices: A hyperconnected analog to the Ruddelsden-Popper structure