Nonadiabatic Multielectron Dynamics in Strong Field Molecular Ionization | Zendy

M. Lezius | Zendy; Valérie Blanchet | Zendy; D. M. Rayner | Zendy; D. M. Villeneuve | Zendy; Albert Stolow | Zendy; Misha Ivanov | Zendy

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Nonadiabatic Multielectron Dynamics in Strong Field Molecular Ionization

Author(s) -

M. Lezius,

Valérie Blanchet,

D. M. Rayner,

D. M. Villeneuve,

Albert Stolow,

Misha Ivanov

Publication year - 2001

Publication title -

physical review letters

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 3.688

H-Index - 673

eISSN - 1079-7114

pISSN - 0031-9007

DOI - 10.1103/physrevlett.86.51

Subject(s) - polyatomic ion , ionization , excitation , fragmentation (computing) , atomic physics , physics , molecular dynamics , molecule , ion , molecular physics , quantum mechanics , computer science , operating system

We report the observation of a general strong field ionization mechanism due to highly nonadiabatic multielectron excitation dynamics in polyatomic molecules. We observe that such excitation mechanisms greatly affect molecular ionization, fragmentation, and energetics. We characterized this phenomenon as a function of optical frequency, intensity, and molecular properties.

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