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Spatial Coherence in Near-Field Raman Scattering
Author(s) -
Ryan Beams,
Luiz Gustavo Cançado,
SangHyun Oh,
Ado Jório,
Lukáš Novotný
Publication year - 2014
Publication title -
physical review letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 3.688
H-Index - 673
eISSN - 1079-7114
pISSN - 0031-9007
DOI - 10.1103/physrevlett.113.186101
Subject(s) - physics , coherence (philosophical gambling strategy) , phonon , raman spectroscopy , raman scattering , scattering , inelastic scattering , field (mathematics) , spectroscopy , x ray raman scattering , optics , incoherent scatter , light scattering , spatial coherence , measure (data warehouse) , condensed matter physics , quantum mechanics , mathematics , pure mathematics , database , computer science
Inelastic light scattering in crystals has historically been treated as a spatially incoherent process, giving rise to incoherent optical radiation. Here we demonstrate that Raman scattering can be spatially coherent, in which case it depends on the dimensionality and symmetry of the scatterer. Using near-field spectroscopy, we measure a correlation length of ∼30  nm for the optical phonons in graphene, the results varying with vibrational symmetries and spatial confinement of the phonons.

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