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X-Ray Second Harmonic Generation
Author(s) -
S. Shwartz,
M. Fuchs,
J. B. Hastings,
Yuichi Inubushi,
Tetsuya Ishikawa,
Tetsuo Katayama,
David A. Reis,
Takahiro Sato,
Kensuke Tono,
Makina Yabashi,
Shimon Yudovich,
S. E. Harris
Publication year - 2014
Publication title -
physical review letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 3.688
H-Index - 673
eISSN - 1079-7114
pISSN - 0031-9007
DOI - 10.1103/physrevlett.112.163901
Subject(s) - high harmonic generation , wavelength , physics , optics , quadratic growth , second harmonic generation , harmonic , laser , radiation , nonlinear optics , phase matching , atomic physics , electron , nonlinear system , phase (matter) , harmonics , diamond , materials science , quantum mechanics , voltage , mathematical analysis , mathematics , composite material
We report clear experimental evidence for second harmonic generation at hard x-ray wavelengths. Using a 1.7 Å pumping beam generated by a free electron laser, we observe second harmonic generation in diamond. The generated second harmonic is of order 10 times the background radiation, scales quadratically with pump pulse energy, and is generated over a narrow phase-matching condition. Of importance for future experiments, our results indicate that it is possible to observe nonlinear x-ray processes in crystals at pump intensities exceeding 1016  W/cm2.

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