Shear Melting of a Colloidal Glass
Author(s) -
Christoph Eisenmann,
Chan-Joong Kim,
Johan Mattsson,
David A. Weitz
Publication year - 2010
Publication title -
physical review letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 3.688
H-Index - 673
eISSN - 1079-7114
pISSN - 0031-9007
DOI - 10.1103/physrevlett.104.035502
Subject(s) - materials science , shear (geology) , mean squared displacement , colloid , gaussian , shear flow , shear rate , colloidal particle , length scale , thermodynamics , optics , rheology , physics , mechanics , composite material , chemistry , molecular dynamics , quantum mechanics
We use confocal microscopy to explore shear melting of colloidal glasses, which occurs at strains of approximately 0.08, coinciding with a strongly non-Gaussian step size distribution. For larger strains, the particle mean square displacement increases linearly with strain and the step size distribution becomes Gaussian. The effective diffusion coefficient varies approximately linearly with shear rate, consistent with a modified Stokes-Einstein relationship in which thermal energy is replaced by shear energy and the length scale is set by the size of cooperatively moving regions consisting of approximately 3 particles.
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