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Extra sub-Doppler lines in the vicinity of the third-resonance 6S-8Ptransition of atomic Cs attributed to optically induced Cs dimers
Author(s) -
Thierry Passerat de Silans,
Isabelle Maurin,
Athanasios Laliotis,
P. Chaves de Souza Segundo,
Daniel Bloch
Publication year - 2011
Publication title -
physical review a
Language(s) - English
Resource type - Journals
eISSN - 1094-1622
pISSN - 1050-2947
DOI - 10.1103/physreva.83.043402
Subject(s) - lambda , physics , resonance (particle physics) , doppler effect , atomic physics , excitation , spectral line , spectroscopy , atom (system on chip) , optics , quantum mechanics , computer science , embedded system
International audienceWe report on the observation of extra sub-Doppler lines in a saturated absorption experiment when exploring the vicinity of the 6S1/2 8P3/2 transition of Cs ( = 388 nm). These extra lines are observed only under a relatively strong irradiation of both the pump and the probe beams. Extra narrow lines are also observed in co-propagating nonlinear spectroscopy, and around the lines of the V-type three-level system 8P3/2 - 6S1/2 - 8P1/2 (1 = 388 nm, 2 = 389 nm). We attribute theses extra-lines to a probing of high-lying molecular caesium, produced as a result of the optical excitation of Cs atoms, as the low Cs atom density ( 1012cm-3) is unable to populate significantly the dimer states in the condition of thermal equilibrium

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