Synthesis and photocatalytic activity of mesoporous g-C 3 N 4 /MoS 2 hybrid catalysts
Author(s) -
Yirong Qi,
Qinghua Liang,
Ruitao Lv,
Wanci Shen,
Feiyu Kang,
ZhengHong Huang
Publication year - 2018
Publication title -
royal society open science
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.84
H-Index - 51
ISSN - 2054-5703
DOI - 10.1098/rsos.180187
Subject(s) - photocatalysis , mesoporous material , graphitic carbon nitride , materials science , catalysis , degradation (telecommunications) , heterojunction , charge carrier , nanotechnology , visible spectrum , chemical engineering , irradiation , optoelectronics , computer science , chemistry , physics , organic chemistry , engineering , telecommunications , nuclear physics
The key to solving environmental and energy issues through photocatalytic technology requires highly efficient, stable and eco-friendly photocatalysts. Graphitic carbon nitride (g-C 3 N 4 ) is one of the most promising candidates except for its limited photoactivity. In this work, a facile and scalable one-step method is developed to fabricate an efficient heterostructural g-C 3 N 4 photocatalyst in situ coupled with MoS 2 . The strong coupling effect between the MoS 2 nanosheets and g-C 3 N 4 scaffold, numerous mesopores and enlarged specific surface area helped form an effective heterojunction. As such, the photocatalytic activity of the g-C 3 N 4 /MoS 2 is more than three times higher than that of the pure g-C 3 N 4 in the degradation of RhB under visible light irradiation. Improvement of g-C 3 N 4 /MoS 2 photocatalytic performance is mainly ascribed to the effective suppression of the recombination of charge carriers.
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