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Metal-free C60/CNTs/g-C3N4ternary heterostructures: synthesis and enhanced visible-light-driven photocatalytic performance
Author(s) -
Xue Lin,
Rui Zhao,
Xi Yang,
Xiangyu Li,
Junyou Shi,
Ning Yan
Publication year - 2018
Publication title -
royal society open science
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.84
H-Index - 51
ISSN - 2054-5703
DOI - 10.1098/rsos.172290
Subject(s) - photocatalysis , rhodamine b , materials science , visible spectrum , ternary operation , heterojunction , catalysis , carbon nanotube , metal , chemical engineering , adsorption , substrate (aquarium) , specific surface area , degradation (telecommunications) , nanotechnology , photochemistry , optoelectronics , chemistry , organic chemistry , metallurgy , telecommunications , computer science , engineering , programming language , oceanography , geology
A metal-free C 60 /CNTs/g-C 3 N 4 nanoheterostructure with excellent visible-light photocatalysis for rhodamine B (Rh B) degradation has been reported. Via a convenient low-temperature solution-phase method, g-C 3 N 4 nanosheets can serve as substrate for dispersion of C 60 /CNTs. The loading of C 60 /CNTs onto g-C 3 N 4 nanosheets surfaces significantly enhanced visible-light-driven photocatalytic activity of g-C 3 N 4 catalyst, for oxidation of organic pollutant (Rh B, 100%). Excellent photocatalytic properties of C 60 /CNTs/g-C 3 N 4 can be predominantly attributed to the intimate interfacial contact among constructing compounds, increased specific surface area and enhanced light adsorption efficiency resulted from C 60 /CNTs carbon materials. Particularly, the synergistic heterostructure interaction remarkably hinders the electron–hole pairs recombination, giving rise to significantly enhanced photocatalytic performance of C 60 /CNTs/g-C 3 N 4 in comparison with other counterparts.

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