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In a laboratory investigation using tunable picosecond lasers in a pump-probe configuration, lifetimes of the E (II)-I-1, v = O and v = 1 states of CO are experimentally determined. For E (II)-I-1, v = 1, the lifetime is found to vary significantly for the isotopomers. Combining the data with existing oscillator strengths, predissociation probabilities within the range of 93.6%-98.64% result for (CO)-C-12-O-16, (CO)-C-13-O-16, and (CO)-C-13-O-18 in, the case of the E (II)-I-1, v=1 state, which is the state that predominantly influences the isotopic fractionation of CO in interstellar clouds.

astrophysical journal/the astrophysical journal

Lifetime Measurements of the [ITAL]E[/ITAL] [TSUP]1[/TSUP]Π, [FORMULA][F]v=0[/F][/FORMULA] and [FORMULA][F]v=1[/F][/FORMULA] States of [TSUP]12[/TSUP]C[TSUP]16[/TSUP]O, [TSUP]13[/TSUP]C[TSUP]16[/TSUP]O, and [TSUP]13[/TSUP]C[TSUP]18[/TSUP]O