Inducing conductivity in polycrystalline ZnO1-x thin films through space charge doping
Author(s) -
Andrea Paradisi,
Johan Biscaras,
Abhay Shukla
Publication year - 2017
Publication title -
journal of applied physics
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.699
H-Index - 319
eISSN - 1089-7550
pISSN - 0021-8979
DOI - 10.1063/1.5001127
Subject(s) - materials science , doping , condensed matter physics , space charge , conductivity , semiconductor , charge carrier , crystallite , thin film , electrical resistivity and conductivity , wide bandgap semiconductor , weak localization , band gap , surface conductivity , depletion region , optoelectronics , electron , nanotechnology , chemistry , physics , magnetoresistance , magnetic field , quantum mechanics , metallurgy
International audienceWe induce ultra-high carrier charge density in polycrystalline zinc oxide thin films on glass with a thickness of few tens of nm, achieving carrier concentrations as high as 2.2×1014cm−2, well beyond the Ioffe-Regel limit for an insulator-metal transition in two dimensions. The sheet resistance is consequently lowered by up to 5 orders of magnitude to about 2 k Ω/◻ without alteration of transparency thanks to our space charge doping technique. Electrostatic doping of such a large band-gap semiconductor is quite challenging, and a high surface potential is required in order to induce conductivity at the interface. Through magneto-transport measurements performed at low temperature on the doped films, we show that both weak localization and weak anti-localization of charge carriers can be observed and that these quantum interference phenomena can be modulated by the carrier concentration and temperature
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