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Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3
Author(s) -
M. Kozina,
Tim van Driel,
Matthieu Chollet,
Takahiro Sato,
James M. Glownia,
Scott Wandel,
M. Radović,
U. Staub,
Matthias C. Hoffmann
Publication year - 2017
Publication title -
structural dynamics
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.415
H-Index - 29
ISSN - 2329-7778
DOI - 10.1063/1.4983153
Subject(s) - terahertz radiation , ultrashort pulse , diffraction , softening , fourier transform , materials science , optics , condensed matter physics , physics , laser , quantum mechanics , composite material
We use ultrafast X-ray pulses to characterize the lattice response of SrTiO 3 when driven by strong terahertz fields. We observe transient changes in the diffraction intensity with a delayed onset with respect to the driving field. Fourier analysis reveals two frequency components corresponding to the two lowest energy zone-center optical modes in SrTiO 3 . The lower frequency mode exhibits clear softening as the temperature is decreased while the higher frequency mode shows slight temperature dependence.

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