Ultrafast X-ray diffraction probe of terahertz field-driven soft mode dynamics in SrTiO3
Author(s) -
M. Kozina,
Tim van Driel,
Matthieu Chollet,
Takahiro Sato,
James M. Glownia,
Scott Wandel,
M. Radović,
U. Staub,
Matthias C. Hoffmann
Publication year - 2017
Publication title -
structural dynamics
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.415
H-Index - 29
ISSN - 2329-7778
DOI - 10.1063/1.4983153
Subject(s) - terahertz radiation , ultrashort pulse , diffraction , softening , fourier transform , materials science , optics , condensed matter physics , physics , laser , quantum mechanics , composite material
We use ultrafast X-ray pulses to characterize the lattice response of SrTiO 3 when driven by strong terahertz fields. We observe transient changes in the diffraction intensity with a delayed onset with respect to the driving field. Fourier analysis reveals two frequency components corresponding to the two lowest energy zone-center optical modes in SrTiO 3 . The lower frequency mode exhibits clear softening as the temperature is decreased while the higher frequency mode shows slight temperature dependence.
Accelerating Research
Robert Robinson Avenue,
Oxford Science Park, Oxford
OX4 4GP, United Kingdom
Address
John Eccles HouseRobert Robinson Avenue,
Oxford Science Park, Oxford
OX4 4GP, United Kingdom