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Cellulose nanocrystals in water suspensions behave as lyotropic liquid crystals forming achiral nematicphase above a critical concentration. Such an organization can be retained in solid filmsand give rise to an intense colored appearance. Here, we characterize their opticalresponse by applying optical and scanning electron microscopy, imaging scatterometry, andangle-resolved reflectance measurements. We show that the experimental results are wellexplained by computational modeling using the finite-difference time-domain method, but slightly lesswell by Berremann’s analytical model

Invited Article: Chiral optics of helicoidal cellulose nanocrystal films