Seed layer technique for high quality epitaxial manganite films
Author(s) -
Patrizio Graziosi,
Alessandro Gambardella,
Marco Calbucci,
Kerry J. O’Shea,
Donald A. MacLaren,
Alberto Riminucci,
I. Bergenti,
Silvio Fugattini,
M. Prezioso,
N. Homonnay,
G. Schmidt,
D. Pullini,
D. Busquets-Mataix,
V. Dediu
Publication year - 2016
Publication title -
aip advances
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.421
H-Index - 58
ISSN - 2158-3226
DOI - 10.1063/1.4961228
Subject(s) - manganite , epitaxy , materials science , substrate (aquarium) , ferromagnetism , layer (electronics) , thin film , optoelectronics , strain engineering , deposition (geology) , condensed matter physics , nanotechnology , silicon , geology , paleontology , oceanography , physics , sediment
We introduce an innovative approach to the simultaneous control of growth mode and magnetotransport properties of manganite thin films, based on an easy-to-implement film/substrate interface engineering. The deposition of a manganite seed layer and the optimization of the substrate temperature allows a persistent bi-dimensional epitaxy and robust ferromagnetic properties at the same time. Structural measurements confirm that in such interface-engineered films, the optimal properties are related to improved epitaxy. A new growth scenario is envisaged, compatible with a shift from heteroepitaxy towards pseudo-homoepitaxy. Relevant growth parameters such as formation energy, roughening temperature, strain profile and chemical states are derived.
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